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The comedown from one No-Doz is much much much worse than a comedown from a few cups of coffee. I've never tried any other caffeine pills besides No-Doz (don't anymore), but when I used to take one in the morning to wake me up, by about 12:30-1:00pm I was ready to crash in the nearest open space. When I comedown from drinking coffee I just get a little drowsy, but usually make it through the rest of the day okay (or just pick up another cup of coffee ).
Stick to the natural stimulants 
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